Entropies of Condensed Phases and Complex Systems: A First Principles Approach by Christian Spickermann (Paperback, 2013)

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Currently, a straightforward calculation of thermodynamic properties from these methods is only possible for high-temperature and low- density systems. Although the enthalpy of a system can often be predicted to a good level of precision with this ideal gas approach, calculating the entropy contribution to the free energy is problematic, especially as the density of the system increases.